Metasurface: a spacer between nanoparticle and back-mirror enhanced the second harmonic generation by ~1000 times

Metasurface: a spacer between nanoparticle and back-mirror enhanced the second harmonic generation by ~1000 times

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Published

  (School of Materials and Chemical Technology / Dr. Saulius Juodkazis)

“Second Harmonic Generation from Phase-Engineered Metasurfaces of Nanoprisms”

MicromachinesDOI:10.3390/mi11090848

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<Abstract>

Metasurfaces of gold (Au) nanoparticles on a SiO2-Si substrate were fabricated for the enhancement of second harmonic generation (SHG) using electron beam lithography and lift-off. Triangular Au nanoprisms which are non-centro-symmetric and support second-order nonlinearity were examined for SHG. The thickness of the SiO2  spacer is shown to be an effective parameter to tune for maximising SHG. Electrical field enhancement at the fundamental wavelength was shown to define the SHG intensity. Numerical modeling of light enhancement was verified by experimental measurements of SHG and reflectivity spectra at the normal incidence. At the plasmonic resonance, SHG is enhanced up to ∼3.5 × 1033 times for the optimised conditions.